Roll-to-roll sputtering equipment FOSA labX  for the deposition of the ZrO2-VO2-ZrO2 layer stack on ultra-thin glass
Energy-saving potential of thermochromic coatings in transparent building envelope components

Authors

  • Matthias Fahland Fraunhofer Institute for Organic Electronics image/svg+xml
  • Jolanta Szelwicka Fraunhofer Institute for Organic Electronics, Electron Beam and Plasma Technology image/svg+xml
  • Wiebke Langgemach Fraunhofer Institute for Organic Electronics, Electron Beam and Plasma Technology image/svg+xml

Downloads

DOI:

https://doi.org/10.47982/jfde.2023.2.A5

Keywords:

smart coatings, energy saving, radiative cooling, smart windows, electrochromic coatings, thermochromic coatings, energy efficiency, vanadium oxide

Abstract

Advances in the energy management of buildings are essential for reducing the carbon footprint in the building sector. Applying special window coatings of varying optical properties offers new chances for improved energy efficiency. Thermochromic vanadium oxide (VO2) is an important material for this development and is, therefore, one of the most investigated thermochromic materials. It changes its transmittance in the infrared spectral range in response to a changing temperature. In this study, VO2 coating was deposited on ultra-thin flexible glass in a continuous roll-to-roll sputtering process. The thermochromic layer had a thickness of 70 nm, and it was embedded between two zirconium oxide layers of 170 nm each. The luminous transmittance of the stack was 50%. A solar modulation of 9.6% was reached between the low and high-temperature states. The transition temperature between the cold infrared transparent and the warm infrared opaque state was determined to be 22°C. Different application scenarios for this material were evaluated. The modulation of the solar transmittance was calculated for the combination of VO2 with state-of-the-art low-e coatings. Our findings show that such a combination does not offer a benefit for reducing the energy demand of a building. However, a stand-alone implementation of thermochromic coatings has a high potential if the energy consumption of the building is dominated by cooling demands.

How to Cite

Fahland, M., Szelwicka, J., & Langgemach, W. (2023). Energy-saving potential of thermochromic coatings in transparent building envelope components. Journal of Facade Design and Engineering, 11(2), 197–210. https://doi.org/10.47982/jfde.2023.2.A5

Published

2023-12-23

References

Algarni, S., Nutter, D. (2015). Survey of Sky EffectiveTemperature Models Applicable to Building Envelope Radiant Heat Transfer. DOI: 10/13140RG.2.1.4212.5526

Aburas, M., Soebarto, V., Wiliamson, T., Liang, R., Ebenhoff-Heidepriem, H., Wu, Y. (2019). Thermochromic smart window technologies for building application: a review. Applied Energy, 255, 113522 DOI: https://doi.org/10.1016/j.apenergy.2019.113522

Bahlawane, N., Lenoble, D. (2014). Vanadium oxide compounds: structure, properties, and growth from the gas phase. Chem. Vap. Deposition, 20, 299–311. DOI: 10.1002/cvde.201400057 DOI: https://doi.org/10.1002/cvde.201400057

Baldassarri, C., Shehabi, A., Asdrubali, F., Masanet, E. (2016). Energy and emissions analysis of Next Generation Electrochromic Devices. SOLAR ENERGY MATERIALS AND SOLAR CELLS 156; p. 170-181. JRC95247 DOI: https://doi.org/10.1016/j.solmat.2015.12.017

Butt, A., de Vries, S., Loonen, R., Hensen, J., Stuiver, A., van den Ham, J., Erich, B. (2021). Investigating the energy saving potential of thermochromic coatings on building envelopes. Applied Energy Volume 291, 116788 DOI: https://doi.org/10.1016/j.apenergy.2021.116788

Chang, T., Coa, X., Bao, S., Ji, S., Luo, H., Jin, P. (2016). Review on thermochromic vanadium dioxide based smart coatings: from lab to commercial application, Adv. Manuf. , 6:1–19, doi.org/10.1007/s40436-017-0209-2 DOI: https://doi.org/10.1007/s40436-017-0209-2

Crosby, P., Netravali, A. (2023). Green Thermochromic Materials: A Brief Review. Advances Sustainable Systems (Vol. 6, Issue 9) 2022, 2200208 https://doi.org/10.1002/adsu.202200208 DOI: https://doi.org/10.1002/adsu.202200208

D’Agostino, D., Mazzarella, L. (2019). What is a Nearly zero energy building? Overview, implementation and comparison of definitions. Journal of Building Engineering, Volume 21, Pages 200-212 DOI: https://doi.org/10.1016/j.jobe.2018.10.019

EN 673:2011, Glass in building - Determination of thermal transmittance (U value) - Calculation method

Gudmundsson, J. T., Brenning, N., Lundin, D., Helmersson, U. (2012). High power impulse magnetron sputtering discharge. Journal of Vacuum Science & Technology A 30, 030801 DOI: https://doi.org/10.1116/1.3691832

Houska, J., Kolenaty, D., Vlcek, J., Barta, T., Rezek, J., Cerstvy, R. (2019). Significant improvement of the performance of ZrO2/V1-xWxO2/ZrO2 thermochromic coatings by utilizing a second-order interference. Solar Energy Materials and Solar Cells 191, 365–371 DOI: https://doi.org/10.1016/j.solmat.2018.12.004

Hu, P., Vu, T. D., Li, M., Wanh, S., Ke, Y., Zeng, X., Mai, L., Long, Y. (2023). Vanadium Oxide: Phase diagrams, Structures, Synthesis and Applications. Chem. Rev., 123, 4353-4415 DOI: https://doi.org/10.1021/acs.chemrev.2c00546

ISO 9050, Glass in building – Determination of light transmittance, solar direct transmittance, total solar energy transmittance, ultraviolet transmittance and related glazing factors

Jelle, B.P. (2013). Solar radiation glazing factors for window panes, glass structures and electrochromic windows in buildings—Measurement and calculation. Solar Energy Materials and Solar Cells, Volume 116, September 2013, Pages 291-323 DOI: https://doi.org/10.1016/j.solmat.2013.04.032

Jin, P., Nakao, S., Tanemura, S. (1998). Tungsten doping into vanadium dioxide thermochromic films by high-energy ion implantation and thermal annealing. Thin Solid Films, Volume 324, Issues 1–2, Pages 151-158 DOI: https://doi.org/10.1016/S0040-6090(98)00362-9

Li, M., Magdassi, S., Gao, Y., Long, Y. (2017). Hydrothermal Synthesis of VO2: Advantages, Challenges and Prospects for the Application of Energy Efficient Smart Windows. Small, 13, 1701147 DOI: https://doi.org/10.1002/smll.201701147

Mohammad, A., Joshi, K., Rana, D., Ilhom, S., Wells, B., Wills, B., Sinkovic, B., Okyay, A., Biykli, N. (2023). Low-temperature synthesis of crystalline vanadium oxide films using oxygen plasmas. J. Vac Si. Technol. A41, 032405 DOI: https://doi.org/10.1116/6.0002383

Rezek, J., Szelwicka, J., Vlcek, J., Cerstvy, R., Houska, J., Fahland, M., Fahlteich, J. (2022). Transfer of the sputter technique for deposition of strongly thermochromic VO2-based coatings on ultrathin flexible glass to large-scale roll-to-roll device. Surface and Coatings Technology, Volume 442, 25, 128273 DOI: https://doi.org/10.1016/j.surfcoat.2022.128273

Solovyev, A.A., Rabotkin, S.V., Kovsharov, N.F. (2015), Polymer films with multilayer low-E coatings. Materials Science in Semiconductor Processing, Volume 38, Pages 373-380 DOI: https://doi.org/10.1016/j.mssp.2015.02.051

Tällberg, R., Jelle, B., Loonen, R., Gao, T., Hamdy, M. (2016). Comparison of energy saving potential of adaptive and controllable smart windows: A state of the art review and simulation studies of thermochromic, photochromic and electrochromic technologies. Solar Energy Materials and Solar Cells, Volume 200, 109828 DOI: https://doi.org/10.1016/j.solmat.2019.02.041

Teixeira, H., Gomes, M., Rodrigues, A. Pereira, J. (2020). Thermal and visual comfort, energy use and environmental performance of glazing systems with solar control films. Building and Environment, Volume 168, 106474 DOI: https://doi.org/10.1016/j.buildenv.2019.106474

Vlcek, J., Koletany, D., Houska, J., Kozak, T., Cerstvy, R. (2017). Controlled reactive HiPIMS—effective technique for low-temperature (300 °C) synthesis of VO2 films with semiconductor-to-metal transition. J. Phys. D: Appl. Phys. 50 38LT01 DOI: https://doi.org/10.1088/1361-6463/aa8356

Vu, T., Chen, Z., Zeng, X., Jiang, M., Liu, S., Gao, Y., Long, Y. (2019) Physical vapour deposition of vanadium dioxide for thermochromic smart window applications. J. Mater. Chem. C, 7, 2121-2145 DOI: https://doi.org/10.1039/C8TC05014G

Wang, S., Jiang, T., Meng, Y., Yang, R., Tan, G., Long, Y. (2021). Scalable thermochromic smart windows with passive radiative cooling regulation. Science 374, 1501-1504 DOI: https://doi.org/10.1126/science.abg0291

Wang, X., Narayan, I. (2021). Thermochromic Materials for Smart Windows: A State-of-Art Review. S. Front. Energy Res. Sec. Solar Energy Volume 9, doi.org/10.3389/fenrg.2021.800382 DOI: https://doi.org/10.3389/fenrg.2021.800382

Yaşar, Y., Maçka Kalfa, S. (2012). The effects of window alternatives on energy efficiency and building economy in high-rise residential buildings in moderate to humid climates. Energy Conversion and Management, Volume 64, Pages 170-181 DOI: https://doi.org/10.1016/j.enconman.2012.05.023